Претрага
310 items
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Testing the energy value of different types of coal by the method of active thermography
In this paper, coal thermograms are presented and analyzed in order to determine their energy value. Two types of coal of different categories, brown and lignite, were selected for active thermographic imaging. The tested coal samples were processed before measurement so that they are similar in dimensions and have two plane-parallel smooth surfaces. The test samples were "primarily" heated under the same conditions and the process of their cooling was monitored by a thermal camera. "Then" they were cooled ...Stevan Đenadić, Ljubiša Tomić, Vesna Damnjanović, Predrag Jovančić, Dragutin Jovković. "Testing the energy value of different types of coal by the method of active thermography" in 9th International Scientific Conference on Defensive Technologies, Belgrade, Serbia, 15-16 October 2020, The Military Technical Institute (2020)
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Uniaxial compressive strength test before and after standard fire test on rock mass
Stefan Mitrović, Goran Todorović, Bojan Kostić, Milica Mirković-Marjanović, Nikola Božović, Marija Krstić, Aleksandar Erić, Radovan Gospavić, Snežana Ilić, Aleksandar Kijanović (2022)... paper, it is not possible to determine uniaxial compressive strength after standard fire test. Standard fire test showed that the rock is of such composition, it will disintegrate at high temperatures. For tunnel structure, this significant drop in strength after standard fire test is not dangerous ...Stefan Mitrović, Goran Todorović, Bojan Kostić, Milica Mirković-Marjanović, Nikola Božović, Marija Krstić, Aleksandar Erić, Radovan Gospavić, Snežana Ilić, Aleksandar Kijanović. "Uniaxial compressive strength test before and after standard fire test on rock mass" in Fifth symposium of the Macedonian Association for Geotechnics, Ohrid, North Macedonia, 23-25. 06. 2022, Macedonian Association for Geotechnics (2022)
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Određivanje zbijenosti starog komunalnog otpada
Bez obzira na savremene tretmane komunalnog otpada u svetu, u Srbiji je i dalje najčešći vid odlaganja na komunalne deponije, pa zbijanje otpada predstavlja jednu od ključnih faza formiranja deponije. Na ovaj način znatno se smanjuje zapremina otpada, ubrzava proces degradacije i produžava radni vek deponije. Zbog toga su geotehničke karakteristike komunalnog otpada prilikom zbijanja, veoma bitne kako u fazi projektovanja tako i u fazi izgradnje deponije i optimizacije prostora. Tu se pre svega misli na maksimalnu suvu zapreminsku ...Jovana Janković, Dragoslav Rakić, Irena Basarić Ikodinović, Tina Đurić. "Određivanje zbijenosti starog komunalnog otpada" in Konferencija Otpadne vode, komunalni čvrsti otpad i opasan otpad, 16-18.06.2021., Beograd : Udruženje za tehnologiju vode i sanitarno inženjerstvo (2021)
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Dehydroicetexanes in sediments and crude oils: Possible markers for Cupressoideae
Hans Peter Nytoft, Geir Kildahl-Andersen, Sofie Lindström, Frode Rise, Achim Bechtel, Danica Mitrović, Nataša Đoković, Dragana Životić, Ksenija A. Stojanović (2019)Two previously unidentified dehydroabietane isomers were isolated from Miocene Serbian lignite and Rhaetian (Late Triassic) coaly mudstones from South Sweden and characterized using NMRspectroscopy as cis- and trans-dehydroicetexane. Both have a 9(10?20)-abeo-abietane or icetexane skeleton, consisting of a 6-7-6 tricyclic framework with seven carbons in ring B instead of the usual six in common diterpanes of the abietane-type. Dehydroicetexanes can be detected using GC-MS-MS in m/z 270?146 chromatograms without interference from dehydroabietane or other isomers. Dehydroicetexanes are often abundant ...Hans Peter Nytoft, Geir Kildahl-Andersen, Sofie Lindström, Frode Rise, Achim Bechtel, Danica Mitrović, Nataša Đoković, Dragana Životić, Ksenija A. Stojanović. "Dehydroicetexanes in sediments and crude oils: Possible markers for Cupressoideae" in Organic Geochemistry, Elsevier BV (2019). https://doi.org/10.1016/j.orggeochem.2019.01.001
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Mineral Resources of Serbia: Environmental, Societal and Economic Challenges
... onal companies. AlI the fatty acid chains incorporated in the biodiesel composition are those originated from the starting triglycerides. Hence, the FAME composition of biodiesel reflects the fatty acid (FA) composition of the source triglycerides and it determines some critical properties of ...
... in linseed is followed regardless of ecological conditions; therefore, the qualitative and quantitative triglyceride composition reflects the differences in fatty acid composition of linseed oil. Linseed oil is an edible oil, and as a nutritional supplement, a source of a-Linolenic acid. Distinctive ...
... Miladinović et al. 2008). Both crops do not have high demands for air temperature in the vegetative phase. Their demand for higher air temperatures increases at the start of the generative phase at the end of June and the first decade in July. The observed mean air temperature in the JJA period ...Vladimir Simić, Rade Jelenković, Dragana Životić. "Mineral Resources of Serbia: Environmental, Societal and Economic Challenges" in Serbia: Current Issues and Challenges in the Areas of Natural Resources, Agriculture and Environment,, Nova Science Publishers, Inc. (2019)
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Polyhedral characteristics of the cosalite-type crystal structures
Sabina Kovač, Predrag Dabić, Aleksandar Kremenović, Aleksandar Pačevski, Ljiljana Karanović, Marko V. Rodić, Martina Tribus (2019)Sabina Kovač, Predrag Dabić, Aleksandar Kremenović, Aleksandar Pačevski, Ljiljana Karanović, Marko V. Rodić, Martina Tribus. "Polyhedral characteristics of the cosalite-type crystal structures" in The Canadian Mineralogist, Mineralogical Association of Canada (2019). https://doi.org/10.3749/canmin.1900017
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Development of a petrographic classification system for organic particles affected by self-heating in coal waste. (An ICCP Classification System, Self-heating Working Group – Commission III)
M. Misz-Kennan, J. Kus, D. Flores, C. Avila, Z. Büçkün, N. Choudhury, K. Christanis, J.P. Joubert, S. Kalaitzidis, A.I. Karayigit, M. Malecha, M. Marques, P. Martizzi, J.M.K. O'Keefe, W. Pickel, G. Predeanu, S. Pusz, J. Ribeiro, S. Rodrigues, A.K. Singh, I. Suárez-Ruiz, I. Sýkorová, N.J. Wagner, D. Životić (2020)Self-heating of coal waste is a major problem in the leading coal-producing and consuming countries, independent of the recent or past coal exploitation history. The phenomenon of self-heating is dependent on many factors such as the properties of organic matter (maceral composition and rank), moisture and pyrite content, climate effects, and storage conditions (shape of the dump or compaction of the coal waste). Once deposited, coal waste undergoes oxidation, which can lead to self- heating with the overall temperatures ...M. Misz-Kennan, J. Kus, D. Flores, C. Avila, Z. Büçkün, N. Choudhury, K. Christanis, J.P. Joubert, S. Kalaitzidis, A.I. Karayigit, M. Malecha, M. Marques, P. Martizzi, J.M.K. O'Keefe, W. Pickel, G. Predeanu, S. Pusz, J. Ribeiro, S. Rodrigues, A.K. Singh, I. Suárez-Ruiz, I. Sýkorová, N.J. Wagner, D. Životić. "Development of a petrographic classification system for organic particles affected by self-heating in coal waste. (An ICCP Classification System, Self-heating Working Group – Commission III)" in International Journal of Coal Geology, Elsevier BV (2020). https://doi.org/10.1016/j.coal.2020.103411
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Influence of DEM resolution on numerical modelling of debris flows in RAMMS - Selanac case study
Debris flows induced by intensive rainfall represent very hazardous phenomena in many parts of the World. Methods for prediction of runout distance of flow like mass movements are different and depending on the input data, rheology, and available or appropriate numerical solution. However, sometimes it is not easy to obtain pre event and post event high-resolution data in the rural or mountainous area. Thus, the topology of terrain is the most important input parameter for the every real case ...... of the flow material can be defined for the resistance of the solid phase (the term containing / which extensively controls deceleration behaviour of a more slowly moving flow. The resistance of the viscous or turbulent fluid phase (the term including / prevails for a more quickly moving flow (Bartelt ...
... contact of Triassic limestones and magmatic rocks with Palaeozoic metamorphic rocks. Debris flow material is highly heterogeneous in lithological composition, as well as grain size distribution (up to m 3 boulders) (Fig. 3). Figure 3 UAV images of a) soure area b) transportation zone (April 2017) ...
... Method One of well used rheological model is Voellmy method (Voellmy, 1955) firstly used in snow avalanche models, which means that is basically one-phase. It is assumed that the initiation mass starts to move as a plug defining shear stress in different points of transportation path. RAMMS DBF software ...Jelka Krušić, Biljana Abolmasov, Mileva Samardžić Petrović. "Influence of DEM resolution on numerical modelling of debris flows in RAMMS - Selanac case study" in 4th Regional Symposium on Landslides in the Adriatic Balkan Region, 23-25 October 2019, Sarajevo, Bosnia and Herzegovina, Geotechnical Society of Bosnia and Herzegovina (2019). https://doi.org/ 10.35123/ReSyLAB_2019
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Пројекат ПРИЗМА: Карактеризација и технолошки поступци за рециклажу и поновну употребу флотацијске јаловине рудника „Рудник“
Владимир Симић, Стефан Петровић, Филип Арнаут, Весна Цветков, Милена Костовић, Драган Радуловић, Јовица Стојановић, Владимир Јовановић, Дејан Тодоровић, Нина Николић, Јелена Сенћански, Грозданка Богдановић, Драгана Мариловић (2024)Владимир Симић, Стефан Петровић, Филип Арнаут, Весна Цветков, Милена Костовић, Драган Радуловић, Јовица Стојановић, Владимир Јовановић, Дејан Тодоровић, Нина Николић, Јелена Сенћански, Грозданка Богдановић, Драгана Мариловић. "Пројекат ПРИЗМА: Карактеризација и технолошки поступци за рециклажу и поновну употребу флотацијске јаловине рудника „Рудник“" in Записници Српског геолошког друштва, Београд : Српско геолошко друштво (2024)
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Demise of the Wetterstein Carbonate Platform and onset of the Dachstein Carbonate Platform recorded in deep-water successions of the East Bosnian-Durmitor megaunit (Pliješevina, northern Montenegro, Dinarides)
Milica Mrdak, Eva Wagerer, Milan Sudar, Nevenka Djerić, Martin Đaković, Hans-Jürgen Gawlick. "Demise of the Wetterstein Carbonate Platform and onset of the Dachstein Carbonate Platform recorded in deep-water successions of the East Bosnian-Durmitor megaunit (Pliješevina, northern Montenegro, Dinarides)" in Geologica Carpathica, Central Library of the Slovak Academy of Sciences (2024). https://doi.org/10.31577/GeolCarp.2023.26
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Kvartarni klastiti iz bušotine kod Aranđelovca (rasadnik Mladost)
Miroslav Radeta (2024)U ovom radu analizirani su kvartarni klastiti iz bušotine kod Aranđelovca IB 18-3, sa ciljem boljeg razumevanja njihovih sedimentoloških i litoloških karakteristika. Kvartarni sedimenti su prilično homogenog/uniformisanog sastava i čine ih finozrni klastiti (dominantno alevroliti) sa određenim procentom peskovite i glinovite frakcije. Oni su iskartirani u samoj povlati i debljina im je 27 m. U podini su gornjokredne karbonatne stene (krečnjaci, laporci, rekristalisali/mermerisani karbonati) i miocenski sediment predstavljeni raznovrsnim varijetetima klastično karbonatnih stena. Ispitivani kvartarni sedimenti odlikuju se odsustvom ...... alming to better understand their sedimentological and lithological characteristics. The Quaternary sediments are fairly homogeneous/uniform in composition, primarily consisting. of fine-grained clastites (dominantly siltstones) with a certain percentage of sandy and clay fractions. These sediments ...
... themselves are of deluvial-proluvial origin. Key words: Quaternary clasts, siltstones, 4randjelovac, granulometry, mineralogical petrographic composition SADRŽAJ J UPOD....aeeaeee e aeeaaeaaeaeaeeaeeaeeeeeeeaeeeeeeaeeeeeeeeeveeeeeeeeeeeeeee 1 PA IJ XOR RRRRIGRRARRRIGIARRRIGIOIRRRRGGOGIGGRROIG ...Miroslav Radeta. Kvartarni klastiti iz bušotine kod Aranđelovca (rasadnik Mladost), 2024
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Sastav i teksture minerala FeO-Fe2O3-TiO2 sistema u vulkanskim stenama i porfirskim ležištima bakra Borske metalogenetske zone
Aleksandar Luković (2021)Proces obrazovanja minerala iz sistema FeO-Fe2O3-TiO2 u uzorcima vulkanskih stena i porfirskih orudnjenja borske zone prikazan kroz pojavu magnetita/hematita i njihovih alteracija. Minerali ove zone su ispitivani optičkim metodama (odbijena i propuštena svetlost), SEM-EDS/BSD, XRPD, LA-ICP-MS metodama. Rezultati ispitivanja su, pored glavnih Fe – Ti oksida, otkrili prisustvo ferijskog ilmenita u hornblenda andezitima I vulkanske faze kao i magnetita sa većim koncetracija Cr u zoni zlotske magnetne anomalije. Ispitivanje uzoraka iz bušotina porfirskih sistema borske zone otkriva postojanje nekoliko ...... disertacija Beograd, 2021 UNIVERSITY OF BELGRADE FACULTY OF MINING AND GEOLOGY Aleksandar D. Luković Composition and textures of the minerals of FeO- Fe2O3-TiO2 system in volcanic rocks and porphyry copper deposits of the Bor metallogenic zone Doctoral ...
... naučna oblast: Fundamentalna i primenjena mineralogija UDK broj: 549.73:553.53(497.11)(043.3). ABSTRACT Composition and textures of the minerals of FeO-Fe2O3-TiO2 system in volcanic rocks and porphyry copper deposits of the Bor metallogenic zone The process ...
... precipitacion from solution and type IIb is alteration product of magnetite in same paragenesis. All types are presented through mineral textures and composition of micro and trace elements. Key words: magnetite, hematite, hemoilmenite, Bor metallogenic zone, porphyry deposits Scientific field: Geosciences ...Aleksandar Luković. Sastav i teksture minerala FeO-Fe2O3-TiO2 sistema u vulkanskim stenama i porfirskim ležištima bakra Borske metalogenetske zone, Beograd : [A. Luković], 2021
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Hydrogeochemistry of Uranium in the Groundwaters of Serbia
Marina Ćuk, Maja Todorović, Petar Papić, Jovan Kovačević, Zoran Nikić. "Hydrogeochemistry of Uranium in the Groundwaters of Serbia" in Uranium - Past and Future Challenges, Springer International Publishing Switzerland (2015). https://doi.org/10.1007/978-3-319-11059-2_89
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Numerical modeling of Selanac debris flow propagation using SPH code
The Selanac debris flow is a very huge event triggered after extreme rainfall caused by Cyclone Tamara activity in the Republic of Serbia in May 2014. The Selanac case study was already modelling in different programs using Voellmy rheology assumptions like RAMMS software. In this paper research are focusing particularly on the process of debris flowing from initiation zone to main deposition area using Geoflow SPH two-phase model considering frictional rheology law. Main rheological parameters are back-calculated using also ...... heterogeneous and multiphase moving mass as a single-phase continuum. The others are considering two phases, solid and liquid, i.e. a granular skeleton with voids filled with either water or mud. If the shear resistance of the fluid phase can be neglected, the stress tensor in the mixture can ...
... calculation of pore water pressures propagation is possible to be obtained using Finite Difference Method coupled with two- phase model. Herein, just results of two-phase model propagation will be presented. The main equations are discussed by Pastor et al. (2009) considering: A. balance of mass ...
... material is highly heterogeneous in lithological SCG-XIII INTERNATIONAL SYMPOSIUM ON LANDSLIDES. CARTAGENA, COLOMBIA- JUNE 15th-19th-2020 composition, as well as grain size distribution (from fines to up to m 3 boulders in volume). The total length of the flow is 1.5 km and width is about ...Jelka Krušić, Biljana Abolmasov, Miloš Marjanović, Manuel Pastor, Saeid M. Tayyebi . "Numerical modeling of Selanac debris flow propagation using SPH code" in SCG-XIII International Symposium on Landslides. Cartagena, Colombia- February 22-26, 2021, International Society for Soil Mechanics And Geotechnical Engineering (2021)
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Integrated Stratigraphy of the Middle–Upper Jurassic of the Krížna Nappe, Tatra Mountains
carbon and oxygen isotopes, radiolarians, calcareous dinoflagellates, radiolarites, Krížna Nappe, West ern Carpathians, Tethys... isotope composition of Oxfordian-Early Kimmeridgian belemnite rostra: palaeo- environmental implications for Late Jurassic seas. Palaeoge- ography, Palaeoclimatology, Palaeoecology, 203: 153—168. Wierzbowski, H., Dembicz, K. & Praszkier, T., 2000. Oxygen and carbon isotope composition of Cal ...
... successions of the Zlic- chov type (Mahe! and Buday, 1968; Michalik, 2007). The Early Jurassic phase of extension gave rise to wide basinal areas and narrow horsts (Plašienka, 2012). A second phase of extension took place during the latest Early Jurassic and resulted in the extensional tilting ...
... an age. These facies pass into Upper Kimmeridgian-Lower Tithonian pelagic carbonates with abundant Saccocoma sp. The bulk-carbonate isotope composition of the carbonate-siliceous deposits shows positive and negative &5C excursions and shifts in the Early Bajocian, Late Bajocian, Early Bathonian ...Renata Jach, Nevenka Đerić, Špela Goričan, Daniela Reháková. "Integrated Stratigraphy of the Middle–Upper Jurassic of the Krížna Nappe, Tatra Mountains" in Annales Societatis Geologorum Poloniae (2014)
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Kinetics, mechanism, and equilibrium studies of the reactions between a ruthenium(II) complex and some nitrogen- and sulfur-donor nucleophiles
Aleksandar M. Mijatović, Ratomir M. Jelić, Jovana Bogojeski, Živadin D. Bugarčić, Biljana Petrović (2013)Kinetika i mehanizam reakcija supstitucije između [Ru(trpi)(bpi)Cl]+ sa nukleofilima gvanozin-5′-monofosfatom, L-histidinom, tioureom i dimetilsulfoksidom proučavani su spektrofotometrijski u 0,1 M NaClO4 na 310 K. Red reaktivnosti za odabrane ligande je: tiourea > gvanozin-5′-monofosfat > L-histidin > DMSO. Ovaj red je povezan sa elektronskim, strukturnim i hemijskim karakteristikama kompleksa i nukleofila. Reakcija supstitucije sa tioureom je proučavana na tri različite temperature (288, 298 i 310 K). Negativna entropija aktivacije DS = potvrđuje asocijativni način aktivacije. Formiranje kompleksa [Ru(trpi)(bpi)H2O]2+ sa ligandima ...... 1493 123 by potentiometric titrations in aqueous 0.1 M NaClO4 at 298 K in concentration ratios of 1:1, 1:2, and 2:1 (metal:- ligand). The composition of the species of the general formula MpHqLr (where M = [Ru(trpy)(bpy)H2O] 2?, HL = 50-GMP or L-His) was calculated using the computer program ...
... mono- functional complex [Ru(trpy)(bpy)Cl]? with 50-GMP and L-His forms very stable products, especially with 50-GMP. Finally, knowledge of the composition and stability of the species in the studied systems, especially at physiological pH, could contribute to a better understanding of some interactions ...Aleksandar M. Mijatović, Ratomir M. Jelić, Jovana Bogojeski, Živadin D. Bugarčić, Biljana Petrović. "Kinetics, mechanism, and equilibrium studies of the reactions between a ruthenium(II) complex and some nitrogen- and sulfur-donor nucleophiles" in Monatshefte für Chemie - Chemical Monthly, Springer Science and Business Media LLC (2013). https://doi.org/10.1007/s00706-013-1044-1
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Influence of mono- and two-component organic modifiers on determination of lipophilicity of tetradentate Schiff bases
Ispitivani su uticaji primene mono- i dvokomponentnih organskih modifikatora na određivanje lipofilnosti 12 tetradentatnih Šifovih baza metodom reverzno-fazne tankoslojne hromatografije. Osnovni cilj je da se proceni tip interakcije između posmatranih jedinjenja i komponenti primenjenih hromatografskih sistema i uspostavi neki obrazac ponašanja kako bi se lakše izabrala kombinacija organskih modifikatora koji će simulirati interakciju u biološkim sistemima na osnovu činjenica da iste osnovne intermolekularne interakcije su odgovorne za ponašanje supstanci i u biološkom i u hromatografskom sistemu. Primenjeni organski modifikator ...Nikola Stevanović, Aleksandar Mijatović, Aleksandar Lolić, Mario Zlatović, Rada Baošić. "Influence of mono- and two-component organic modifiers on determination of lipophilicity of tetradentate Schiff bases" in Chemical Papers, Springer Science and Business Media LLC (2021). https://doi.org/10.1007/s11696-021-01884-5
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Mesozoic carbonate rocks in Serbia used as dimension stone
Vesna Matović, Tijana Vojnović Ćalić (2016)The building industry in Serbia uses, to a great extent, imported natural stone for architectural purposes. The significance of local deposits, particularly limestones, is not adequately perceived despite the country’s abundance of these valuable resources. Therefore, this study focuses on Serbia’s Mesozoic carbonate rocks, specifically on the deposits of four selected quarries: Klisura, Skrzut, Struganik, and Tisnica. The quality and prospects of the application of these limestones has not yet been the subject of a detailed, comprehensive investigation. Therefore, ...... Leica DMLSP microscope for polarized light connected to a Leica DC 300 digital camera. The thin sections were used to determine the mineral composition and microtextural features (size and type of allochem) for the purpose of rock classification, according to Folk (1959) and Flugel (2004). ...
... slightly and is in range of 2,650–2,690 kg/ m* (Fig. 4a). The values of real density (2,700–2,712 kg/ m?) are in accordance with the mineral composition of these almost pure limestones (the main mineral is calcite with a density value of 2,710 kg/m?*; Fig. 4a). The constant real density values ...Vesna Matović, Tijana Vojnović Ćalić. "Mesozoic carbonate rocks in Serbia used as dimension stone" in Bulletin of Engineering Geology and the Environment, Springer Science and Business Media LLC (2016). https://doi.org/10.1007/s10064-015-0722-0
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Mitigating hydrate formation in onshore gas wells: A case study on optimization techniques and prevention
Gas wells, particularly those situated onshore, play a vital role in the global energy sector by supplying a significant portion of natural gas. However, operational challenges, notably gas hydrate formation, pose substantial issues, leading to complications such as flowline blockages and unexpected well shutdowns. Gas hydrates, crystalline structures resembling ice, ...Gas Well, Gas Hydrate Formation, Well Modeling, Well Performance Optimization, Choke Position Adjustments, Methanol InjectionMilica Ješić, Bojan Martinović, Stefan Stančić, Miroslav Crnogorac, Dušan Danilović. "Mitigating hydrate formation in onshore gas wells: A case study on optimization techniques and prevention" in Underground Mining Engineering, Beograd : Rudarsko-geološki fakultet (2023)
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Adsorption and degradation of some psychiatric drugs by sol-gel synthesized titania-based photocatalysts: influence of tungsten and sodium content
Nina L. Finčur, Maja J. Šćepanović, Mirjana Grujić-Brojčin, Biljana F. Abramović, Jugoslav B. Krstić, Aleksandar Kremenović, Tatjana Srećković, Aleksandar Golubović (2019)Mesoporous anatase nanopowders were doped with 0.05−0.5 mol% of W6, in order to obtain more efficient photocatalyst than TiO2 Degussa P25 in the degradation of amitriptyline (AMI) under simulated solar irradiation (SSI). Dominant XRPD peaks were ascribed to anatase phase, with additional peaks which could correspond to brookite, TiO2 bronze and sodium titanate, Na2Ti9O19. The Raman scattering measurements have confirmed anatase as dominant phase, with broad Raman feature at ~270 cm−1 possibly related to Ti–O–Na stretching vibration. All W-doped ...Sol-gel synthesis, Doped titania nanopowders, XRPD, Raman spectroscopy, Adsorption and photocatalytic degradation, Psychiatric drugsNina L. Finčur, Maja J. Šćepanović, Mirjana Grujić-Brojčin, Biljana F. Abramović, Jugoslav B. Krstić, Aleksandar Kremenović, Tatjana Srećković, Aleksandar Golubović. "Adsorption and degradation of some psychiatric drugs by sol-gel synthesized titania-based photocatalysts: influence of tungsten and sodium content" in Journal of Sol-Gel Science and Technology, Springer Science and Business Media LLC (2019). https://doi.org/10.1007/s10971-019-04925-4