Microstructural and magnetic properties of electrospun hematite/cuprospinel composites

Објеката

Тип
Рад у часопису
Верзија рада
објављена верзија
Језик
енглески
Креатор
Mira Ristić, Aleksandar Kremenović, Michael Reissner, Željka Petrović, Svetozar Musić
Извор
Journal of Materials Science: Materials in Electronics
Издавач
Springer Science and Business Media LLC
Датум издавања
2020
Сажетак
Phase composition, microstructural and magnetic properties of electrospun hematite/cuprospinel composites were investigated. Samples were synthesized starting with 0 to 10 mol% of copper relative to iron. The round shape of reference electrospun fbres was preserved upon their heating up to 600 °C in air, whereas at 700 °C hollow substructure was additionally formed. In these reference samples the presence of hematite phase was detected by XRPD. A small amount (traces) of Fe3O4 /γ-Fe2O3 was also found, due to the reduction conditions created during the burning of the polyvinylpyrrolidone matrix. Rietveld analysis of samples containing 10 mol% copper and produced at 500 °C and 700 °C did not show the tendency to form solid solutions between hematite and Cu cations. Electrospun fbres containing 10 mol% copper after heating at 500 °C consisted of magnetite and cubic cuprospinel as the dominant phases and hematite as the associated phase. Upon heating at 700 °C the phase composition showed the presence of hematite as the dominant phase and tetragonal cuprospinel as the associated phase. For this tetragonal cuprospinel the formula Cu0.6Fe2.4O4 was calculated. Mössbauer spectra recorded at 20 °C and at liquid helium temperature also showed the presence of hematite and spinel structures. Measured hyperfne magnetic splitting refected the distributions of Fe2+, Fe3+ and Cu2+ cations in the spinel structures. The magnetic measurements also confrmed that there is no Cu incorporation into the electrospun hematite.
том
31
Број
12
почетак странице
9812
крај странице
9825
doi
10.1007/s10854-020-03526-0
issn
0957-4522
Subject
Electrical and Electronic Engineering, Condensed Matter Physics, Atomic and Molecular Physics and Optics, Electronic, Optical and Magnetic Materials
Шира категорија рада
M20
Ужа категорија рада
М22
Права
Затворени приступ
Лиценца
All rights reserved
Формат
.pdf

Mira Ristić, Aleksandar Kremenović, Michael Reissner, Željka Petrović, Svetozar Musić. "Microstructural and magnetic properties of electrospun hematite/cuprospinel composites" in Journal of Materials Science: Materials in Electronics, Springer Science and Business Media LLC (2020). https://doi.org/10.1007/s10854-020-03526-0

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